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Yokoyama, Tatsunori; Kokubu, Yoko; Murakami, Hiroaki; Hirata, Takafumi*; Sakata, Shuhei*; Danhara, Toru*; Iwano, Hideki*; Chang, Q.*; Kimura, Junichi*
no journal, ,
The chronological information about carbonates is useful for modeling and enables forecast of geological and geochemical environmental changes by simulating. The U-Th-Pb dating method for carbonates which were formed at reducing environment remain to be established. The final goal of our study is to establish in situ U-Th-Pb dating method for carbonates which are filling cracks in pervious rock like fault rocks. In this study, the U-Th-Pb elemental and isotopic two-dimension distribution for an ammonite fossil were visualized by "Imaging" method using Laser-ablation ICP Mass Spectrometry. In U-Pb isotope analysis for carbonates in cracks of granites, we could not obtain significant U-Pb age data by the lack of uranium and influence of non-radiogenic common lead. When the concentration of lead is sufficiently high for the measurement, we obtained reliable isotopic data from carbonates and their lead isotopic composition reflected characteristic composition of their origin water.
Yokoyama, Tatsunori; Kokubu, Yoko; Murakami, Hiroaki; Watanabe, Takahiro; Hirata, Takafumi*; Sakata, Shuhei*; Danhara, Toru*; Iwano, Hideki*; Maruyama, Seiji*; Miyazaki, Takashi*; et al.
no journal, ,
Chronological and geochemical studies of carbonates, which are commonly found as fracture filling minerals in rocks, can provide information about geochemical conditions present during formation including in deep subsurface environments. A dating technique for the carbonates using laser ablation-multiple collector-inductively coupled plasma mass spectrometry (LA-MC-ICPMS) is still immature partly because of a lack of a consensus international carbonate standard for the in-situ dating technique. In this study, we performed a survey on the carbonate standard materials that may be suitable for high precision U-Th-Pb dating using LA-MC-ICPMS. We examined carbonate standard materials JCp-1 and JCt-1 issued by the Geological Survey of Japan (GSJ). Based on solution-based bulk analysis using MC-ICP-MS, heterogeneities in Pb isotope compositions were confirmed. Nevertheless, the 206Pb-based isotopic compositions were all within 1.2 per mill variations acceptable for a standard used for age determination using LA-MC-ICPMS. Additional tests on the heterogenities in U-Th-Pb compositions of the carbonate standards along with determinations of other trace elements using a 2D imaging LA-ICP-MS are ongoing. Examinations on both natural standards and synthetic standards are ongoing for further efforts in determination of the standard suitable for U-Th-Pb dating of carbonates.
Yokoyama, Tatsunori; Kokubu, Yoko; Murakami, Hiroaki; Watanabe, Takahiro; Mitsuguchi, Takehiro
no journal, ,
no abstracts in English
Ishimaru, Tsuneari
no journal, ,
In the Tono Geoscience Center, it has been promoting that the research and development with the aim of standardization and sophistication of the dating method and techniques using the modern analytical instrumentation, as a new name "Toki Research Institute of Isotope Geology and Geochronology" from 2014 November.
Yokoyama, Tatsunori
no journal, ,
no abstracts in English
Ogata, Nobuhisa
no journal, ,
The overview of geochronology at Toki Research Institute of Isotope Geology and Geochronology are given lectures as the invited lectures of the 128th lecture of the Japan Geodetic Society.
Yokoyama, Tatsunori; Mitsuguchi, Takehiro; Sueoka, Shigeru
no journal, ,
In recent years, it has become possible to carry out high-precision microscale age dating of geological samples using developed micro-analytical techniques such as SIMS, LA-ICP-MS, etc. Application of LA-ICP-MS-based microscale U-Pb dating is extending from U-rich heavy minerals such as zircon, apatite and monazite to U-depleted minerals such as calcite. This kind of method enables age determination of several types of mineral grains occurring within rock bodies, and thereby reveals chronological changes in chemical composition of source materials from which the minerals were crystallized, with some cases in which thermal history of the crystal formation system can be reconstructed. For research and development of geological disposal techniques for high-level radioactive wastes, we develop and facilitate geochronological dating techniques for evaluation of long-term stability in geological environments, at Tono Geoscience Center, Japan Atomic Energy Agency. In our presentation, we introduce the current status of our development for research on long-term stability of geological environments, U-Pb dating of calcite, U-Pb dating of young zircon and trace element analysis by using LA-ICP-MS.
Shimada, Koji
no journal, ,
This report describes the current status of the development of dating technology at the Tono Geoscience Center, provides an overview of the significance of dating, and a framework of dating techniques, and highlights some of the achievements and current challenges.